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"I'm lucky to be in this, and I'm sure Audrey Hepburn felt the same," the UN Goodwill Ambassador told US host Ann Curry.
The late Breakfast At Tiffany's star, who was also a Goodwill Ambassador for the UN, spent almost 40 years helping impoverished children around the world until her death in 1993, and was awarded with the Presidential Medal of Freedom for her work in 1992.
"She was the fortunate one to be able to meet all those kids around the world," Angelina explains.
"You know, we're just in a very fortunate situation that we get to be able to give a voice to these extraordinary people."
Angelina hopes to continue her work with the organisation and the refugees.
"There's been refugees since the dawn of time. And I'm sure, you know, my children will be visiting and learning from refugees in the future."